Novel and efficient base-mediated N-alkylation and amidation of amidines with alcohols have been developed, which can be carried out in one-pot reaction conditions, which allows for the synthesis of a wide range of N-alkyl amines and free amides in good to excellent yields with high atom economy. These metrics are regularly updated to reflect usage leading up to the last few days. . Cooperative Mn( Find more information on the Altmetric Attention Score and how the score is calculated. Selectivity Control in Catalytic Reductive Amination of Furfural to Furfurylamine on Supported Catalysts. Control of Absolute Stereochemistry in Transition‐Metal‐Catalysed Hydrogen‐Borrowing Reactions. N ii - and Catalytic Asymmetric Synthesis of Cyclohexanes by Hydrogen Borrowing Annulations. ]pyrimidines from Acceptorless and Base‐Free Dehydrogenation of Alcohols Mediated by a Dipyridylamine‐Iridium(III) Catalyst. Recent advances of producing Bio-based N-containing compounds via thermo-chemical conversion with ammonia process. The Supporting Information is available free of charge at Journal of Labelled Compounds and Radiopharmaceuticals. Information. Enter your email address below and we will send you your username, If the address matches an existing account you will receive an email with instructions to retrieve your username, By continuing to browse this site, you agree to its use of cookies as described in our, I have read and accept the Wiley Online Library Terms and Conditions of Use. Working off-campus? In water alkylation of amines with alcohols through a borrowing hydrogen process catalysed by ruthenium nanoparticles. Manganese(I)-Catalyzed Cross-Coupling of Ketones and Secondary Alcohols with Primary Alcohols. Users are In particular, the recent progress applying organometallic catalysts based on iridium, ruthenium, and other metals will be discussed. p Homogeneous cobalt-catalyzed reductive amination for synthesis of functionalized primary amines. N One-pot conversion of lysine to caprolactam over Ir/H-Beta catalysts. Key Laboratory of Sensor Analysis of Tumor Marker, Ministry of Education, Shandong Key Laboratory of Biochemical Analysis, Key Laboratory of Analytical Chemistry for Life Science in Universities of Shandong, College of Chemistry and Molecular Engineering, Qingdao University of Science and Technology, Qingdao 266042, P. R. China, Shandong Provincial Key Laboratory of Molecular Engineering, School of Chemistry and Pharmaceutical Engineering, Qilu University of Technology (Shandong Academy of Sciences), Jinan 250014, P. R. China, Co-Innovation Center of Efficient Processing and Utilization of Forest Resources, Nanjing Forestry University, Nanjing 210037, P. R. China, Base-Mediated Amination of Alcohols Using Amidines. Cyano-borrowing: titanium-catalyzed direct amination of cyanohydrins with amines and enantioselective examples. -CH -CD Please check your email for instructions on resetting your password. Please note: If you switch to a different device, you may be asked to login again with only your ACS ID. Heterocycles via Cross Dehydrogenative Coupling. Compared to other synthetic methodologies for the synthesis of amines, these transformations are highly attractive because often alcohols are readily available starting materials, some of them on a large scale from renewable sources. Cp*Co( A nanoscale iron catalyst for heterogeneous direct A practical base mediated synthesis of 1,2,4-triazoles enabled by a deamination annulation strategy. Plasma‐Made (Ni0.5Cu0.5)Fe2O4 Nanoparticles for Alcohol Amination under Microwave Heating. Electronic Supporting Information files are available without a subscription to ACS Web Editions. Promotional Effect of Cu for Catalytic Amination of Diethylene Glycol with Tertiarybutylamine over Ni–Cu/Al2O3 Catalysts. Aza-crown compounds synthesised by the self-condensation of 2-amino-benzyl alcohol over a pincer ruthenium catalyst and applied in the transfer hydrogenation of ketones. . The above reaction was applied to 1-(2,6-dimethylphenoxy)-2-propanol and cyclohexanol. 2 . Ruthenium and Iron‐Catalysed Decarboxylative N‐alkylation of Cyclic α‐Amino Acids with Alcohols: Sustainable Routes to Pyrrolidine and Piperidine Derivatives. Rational Optimization of Lewis‐Acid Catalysts for Direct Alcohol Amination, Part 2 – Titanium Triflimide as New Active Catalyst. d 5 Pr2O3 Supported Nano‐layered Ruthenium Catalyzed Acceptorless Dehydrogenative Synthesis of 2‐Substituted Quinolines and 1,8‐Naphthyridines from 2‐Aminoaryl Alcohols and Ketones. In the case of 1-(2,6-dimethylphenoxy)-2-propano 1 only the corresponding primary amine with an 80% yield and 2,6-dimethy1phenol as a by-product were obtained. 3 N Organic Preparations and Procedures International. Scalable preparation of stable and reusable silica supported palladium nanoparticles as catalysts for N-alkylation of amines with alcohols. Number of times cited according to CrossRef: Ru/HZSM-5 as an efficient and recyclable catalyst for reductive amination of furfural to furfurylamine.

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